Abstract

Abstract Understanding the hydroclimate representations of precipitation δ18O (δ18Op) in tropical South America (TSA) is crucial for climate reconstruction from available speleothem caves. Our preceding study (Part I) highlights a heterogeneous response in millennial hydroclimate over the TSA during the last deglaciation (20–11 ka before present), characterized by a northwest–southeast (NW–SE) dipole in both rainfall and δ18Op, with opposite signs between central-western Amazon and eastern Brazil. Mechanisms of such δ18Op dipole response are further investigated in this study with the aid of moisture tagging simulations. In response to increased meltwater discharge, the intertropical convergence zone (ITCZ) migrates southward, causing a moisture source location shift and depleting the isotopic value of the vapor transported into eastern Brazil, which almost entirely contributes to the δ18Op depletion in eastern Brazil (SE pole). In contrast, the moisture source location change and local condensation change (due to the lowering convergence level and increased rain reevaporation in unsaturated subcloud layers) contribute nearly equally to the δ18Op enrichment in the central-western Amazon (NW pole). Therefore, although a clear inverse relationship between δ18Op and rainfall in both dipole regions seems to support the “amount effect,” we argue that the local rainfall amount only partially interprets the millennial δ18Op change in the central-western Amazon, while δ18Op does not document local rainfall change in eastern Brazil. Thus, the paleoclimate community should be cautious when using δ18Op as a proxy for past local precipitation in the TSA region. Finally, we discuss the discrepancy between the model and speleothem proxies on capturing the millennial δ18Op dipole response and pose a challenge in reconciling the discrepancy. Significance Statement We want to comprehensively understand the hydroclimate footprints of δ18Op and the mechanisms of the millennial variability of δ18Op over tropical South America with the help of water tagging experiments performed by the isotope-enabled Community Earth System Model (iCESM). We argue that the millennial δ18Op change in eastern Brazil mainly documents the moisture source location change associated with ITCZ migration and the change of the isotopic value of the incoming water vapor, instead of the local rainfall amount. In contrast, the central-western Amazon partially documents the moisture source location shift and local precipitation change. Our study cautions that one should not simply resort to the isotopic “amount effect” to reconstruct past precipitation in tropical regions without studying the mechanisms behind it.

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