Abstract
The antiphase structure (APS) of CIDEP spectra of spin correlated radical pairs in viscous liquids is investigated theoretically in a free diffusion model for relative motion of radicals. A very simple and accurate for formula for relative APS amplitude is derived. This formula predicts a very small APS amplitude for the radical pair 2 (CH 3) 2ĊOH at T≈ −45°C. The amplitude is two orders of magnitude smaller than the experimental one, suggesting that the free-diffusion-model description of the relative motion of radicals is not correct.
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