Abstract

The potential of producing ecofriendly composites from industrial waste fibres, bonded with magnesium lignosulfonate, a lignin-based formaldehyde-free adhesive, was investigated in this work. Composites were produced in the laboratory using the following parameters: a hot press temperature of 210 °C, a pressing time of 16 min, and a 15% gluing content of magnesium lignosulfonate (on the dry fibres). The physical and mechanical properties of the produced composites were evaluated and compared with the European Standard (EN) required properties (EN 312, EN 622-5) of common wood-based panels, such as particleboards for internal use in dry conditions (type P2), load-bearing particleboards for use in humid conditions (type P5), heavy-duty load-bearing particleboards for use in humid conditions (type P7), and medium-density fibreboards (MDF) for use in dry conditions. In general, the new produced composites exhibited satisfactory mechanical properties: a bending strength (MOR) (18.5 N·mm−2) that was 42% higher than that required for type P2 particleboards (13 N·mm−2) and 16% higher than that required for type P5 particleboards (16 N·mm−2). Additionally, the modulus of elasticity (MOE) of composites (2225 N·mm−2) was 24% higher than that required for type P2 particleboards (1800 N·mm−2) and equivalent to the required MOE of MDF panels for use in dry conditions (2200 N·mm−2). However, these ecofriendly composites showed deteriorated moisture properties, i.e., 24 h swelling and 24 h water absorption, which were a distinct disadvantage. This should be further investigated, as modifications in the lignosulfonate formula used and/or production parameters are necessary.

Highlights

  • Optimisation of resource efficiency is one of the key objectives to implement the principles of circular economy and face the challenges of increased demand for wood and wood-based products worldwide

  • Composites with acceptable physical and mechanical properties according to European Standard (EN), except for thickness swelling, may producedphysical from industrial waste fibres, bonded with a lignin-based

  • Composites withbe acceptable and mechanical properties according to ENs, formaldehyde-free adhesive, namely, magnesium lignosulfonate

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Summary

Introduction

Optimisation of resource efficiency is one of the key objectives to implement the principles of circular economy and face the challenges of increased demand for wood and wood-based products worldwide. Pulp and paper industries generate significant quantities of nonhazardous solid waste and sludge, which require efficient utilisation as waste materials or by-products [3,4]. Conventional adhesive systems used for wood composites are commonly made of fossil-derived constituents, which are based on formaldehyde, urea, phenol, melamine, and/or isocyanates [10,11,12,13]. Due to their high reactivity, chemical versatility, cost effectiveness, and technological performance regarding their strength of adhesion and moisture resistance, formaldehyde-based polycondensation

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