Abstract

Emergence of hierarchy during compression of quasi-planar bilayers is preceded by a mode-locked state during which the quasi-planar form persists. Transition to hierarchy is determined entirely by geometrically observable parameters. This results in a universal transition phase diagram that enables one to deterministically tune hierarchy even with limited knowledge about material properties.

Highlights

  • The MIT Faculty has made this article openly available

  • We have overcome this limitation for the specific case of hierarchical wrinkled patterns by demonstrating deterministic switching of hierarchy during compression of quasi-planar bilayers

  • We show that the emergence of hierarchy during compression of quasi-planar bilayers is determined by two competing effects that arise due to the non-flat periodic geometry of such systems

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Summary

Present address

Several empirical studies have demonstrated the feasibility of hierarchical wrinkle formation by “adding up” patterns.[17,18,19,20,21] Physical pattern addition is often achieved by compressing a pre-patterned non-flat bilayer.[19,20,21] This non-flat geometry can be conveniently generated via recursive wrinkling, that is, by replicating/imprinting wrinkled patterns that are fabricated via compression of flat bilayers.[19] As wrinkled patterns form due to non-linear buckling bifurcation phenomena, the observed composite patterns are not equivalent to a linear superposition of the elementary patterns To predict these composite patterns, approximate semi-empirical models may be generated by reducing the prepatterned system to either a flat bilayer[21] or a curved bilayer with a non-zero average global curvature.[22] such approximations do not capture the physical effect of quasi-planar geometry on pattern formation. Emergence of hierarchy is preceded by a mode-locked state during which the quasiplanar form persists

Results and Discussion
Conclusions
Curing of PDMS Films
Fabrication of Pre-Stretched Bilayers and Wrinkles
Fabrication of Quasi-Planar Base Layers
Metrology Protocol
Finite Element Simulations
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