Determination of the absorption and radiative decay rates of dark and bright plasmonic modes

Abstract

When two degenerate surface plasmon polariton (SPP) modes couple, in addition to the creation of plasmonic band gap, their respective decay rates are modified as well, resulting in the formation of a pair of dark and bright modes. We combine temporal coupled mode theory, finite-difference time-domain simulation, and angle- and polarization-resolved reflectivity spectroscopy to study the absorption and radiative decay rates of this pair in periodic system. One-dimensional metallic groove arrays are served as an example here. We find for arrays with small groove width, when approaching to the coupling of -1 and + 1 SPP modes, while the radiative decay rate of the high energy mode tends to become zero, the absorption rate decreases as well, forming a "cold" dark mode. At the same time, both the absorption and radiative decay rates of the low energy mode increase, yielding a "hot" bright mode. The situation is completely reversed when groove width increases, turning the high energy mode into a "cold" bright mode and vice versa for the low energy mode. We attribute such modifications to the interplay between the real and imaginary parts of the complex coupling constant, which are found to be highly geometry dependent. Further numerical simulations show the hybridized modes exhibits distinctive electric and magnetic field symmetries, giving rise to different surface charge distributions and Poynting vector profiles, which significantly affect the resulting absorption and radiation losses. Finally, we have measured the decay rates and the complex coupling constant of the hybridized modes and the experimental results are consistent with the analytic and numerical results.