Abstract
A flow concept is developed to measure fast gas–liquid reaction kinetics based on a tube-in-tube reactor.
Highlights
The determination of gas–liquid reaction kinetics is often performed with a stirred cell reactor by recording the pressure decay over time with no analysis of the liquid phase.[10,11] This method is simple to operate and widely applied
To demonstrate the accuracy and efficiency of this automated platform for reaction kinetics determination, we considered two case studies: absorption of CO2 into aqueous methyl diethanolamine (MDEA) (Scheme 1) and ozonolysis of propionaldehyde (Scheme 2)
The reaction kinetics of CO2 with aqueous MDEA are well described in the literature using different techniques.[33,34,35]
Summary
The determination of gas–liquid reaction kinetics is often performed with a stirred cell reactor by recording the pressure decay over time with no analysis of the liquid phase.[10,11] This method is simple to operate and widely applied. This model is used to determine the kinetic reaction rate from gas uptake data at various liquid flow rates.
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