Abstract
Stimulated Raman scattering (SRS) has been observed for the first time in a tetragonal LiYbF4 crystal. The recorded Stokes and anti-Stokes components of χ(3) nonlinear lasing are attributed to the two SRS-active phonon modes with ωSRS1 ~ 325 cm–1 and ωSRS2 ~ 432 cm–1 of this crystal.
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