Detecting nonlocality by second-harmonic generation from a graphene-wrapped nanoparticle.

Abstract

With the rapid development of nanofabrication technology and nonlinear optics, the nonlinear detection by nanostructures is highly appreciated. In this paper, we study the second-harmonic generation by a spherical nonlocal plasmonic nanoparticle wrapped with graphene. We develop a simple method for calculating the electric field at second-harmonic frequency and analyze the influence of the nonlocal response of the metal on the second-harmonic. We find that this nanostructure can probe the material's properties by detecting the radiation intensity of the second-harmonic generation. In addition, the nonlocal response of the plasmonic core can promote the absorption efficiency of second-harmonic generation. Our study may offer a new way for studying the plasmonic quantum effects and nonlinear probing technology and improving the nonlinear conversion efficiency of photonic devices.