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Abstract
Detailed modeling of soot particle nucleation and growth in laminar premixed hydrocarbon flames is presented. The model begins with fuel pyrolysis, followed by the formation of polycyclic aromatic hydrocarbons, their planar growth and coagulation into spherical particles, and finally, surface growth and oxidation of the particles. The computational results are in quantitative agreement with experimental results from several laminar premixed hydrocarbon flames. A detailed analysis of soot particle inception and surface growth processes is presented. Surface growth was described in terms of elementary chemical reactions of surface active sites. The density of these sites was found to depend on the chemical environment. The model predicts the classical picture of soot particle inception and the classical description of soot particle structure.
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