Abstract
A series of novel diphenyl ethylenediamine (DPEN) derived C2 symmetric dihydroimidazolium cyclophanes were designed and synthesized as organo NHC precatalysts. The resultant organo NHC-catalyzed reactions with superior enantioselectivity than traditional C2 dihydroimidazolidine NHCs as exemplified by NHC-catalyzed asymmetric intramolecular Stetter reactions.
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