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Abstract
We have studied the time-correlation function associated with depolarized Rayleigh scattering in dilute polymer solution starting from a general expression, we have reduced the time-correlation function of polarizability to two parts: one involving the overall rotation of the whole molecule and the other the local segmental motion modulated by overall rotation. The time-correlation function for segmental motion is expressed in terms of reorientation of chain segments through angles of arbitrary size.
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