Abstract

Quantum dots are arguably the best interface between matter spin qubits and flying photonic qubits. Using quantum dot devices to produce joint spin-photonic states requires the electronic spin qubits to be stored for extended times. Therefore, the study of the coherence of spins of various quantum dot confined charge carriers is important both scientifically and technologically. In this study we report on spin relaxation measurements performed on five different forms of electronic spin qubits confined in the very same quantum dot. In particular, we use all optical techniques to measure the spin relaxation of the confined heavy hole and that of the dark exciton - a long lived electron-heavy hole pair with parallel spins. Our measured results for the spin relaxation of the electron, the heavy-hole, the dark exciton, the negative and the positive trions, in the absence of externally applied magnetic field, are in agreement with a central spin theory which attributes the dephasing of the carriers' spin to their hyperfine interactions with the nuclear spins of the atoms forming the quantum dots. We demonstrate that the heavy hole dephases much slower than the electron. We also show, both experimentally and theoretically, that the dark exciton dephases slower than the heavy hole, due to the electron-hole exchange interaction, which partially protects its spin state from dephasing.

Highlights

  • The electronic spin in semiconductor nanostructures can often be described as an isolated physical two-level system

  • As we show in Appendix B, below, that the dark exciton (DE) nuclear field-induced dephasing is caused mainly due to small DE-bright excitons (BEs) mixing terms

  • The first fast dephasing step is a measure for the strong Fermi-contact hyperfine interaction of the electron with the nuclear spin bath, while the second step measures the strength of the quadrupole interaction of the nuclear spin bath with the strain-induced electric field gradients in the quantum dots (QDs)

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Summary

INTRODUCTION

The electronic spin in semiconductor nanostructures can often be described as an isolated physical two-level system. At low temperatures and in the absence of external magnetic field, the main decoherence mechanism of these electronic spin qubits is the hyperfine interaction between the electronic (central) spin and the spin of the nuclei of the approximately 105 atoms which form the QDs [14,15,16]. A great deal of effort was devoted to study the coherence properties of the central electronic spin for both, conduction-band electrons [36,37,38,39], and valence-band heavy holes [22,40,41,42,43,44,45], confined in QDs. The temporal evolution of a single electron spin at vanishing external magnetic field was experimentally measured recently by Bechtold and co-workers [33].

THE DEVICE AND EXPERIMENTAL METHODS
RESULTS AND DISCUSSION
SUMMARY
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