Defect-driven ferrimagnetism and hidden magnetization in MnBi2Te4

Abstract

MnBi$_2$Te$_4$ (MBT) materials are promising antiferromagnetic topological insulators where field driven ferromagnetism is predicted to cause a transition between axion insulator and Weyl semimetallic states. However, the presence of antiferromagnetic coupling between Mn/Bi antisite defects and the main Mn layer can reduce the low-field magnetization, and it has been shown that such defects are more prevalent in the structurally identical trivial magnetic insulator MnSb$_2$Te$_4$ (MST). We use high-field magnetization measurements to show that the magnetization of MBT and MST occur in stages and full saturation requires fields of~$\sim$~60 Tesla. As a consequence, the low-field magnetization plateau state in MBT, where many determinations of quantum anomalous Hall state are studied, actually consists of ferrimagnetic septuple blocks containing both a uniform and staggered magnetization component.