Abstract
The hyperfine structure in the 1 01 ← 0 00 transitions of H 2O…DF and H 2O…HF arising from D-nuclear quadrupole and H(D), 19F nuclear-spin—nuclear-spin coupling effects have been resolved and measured by the technique of pulsed-nozzle, Fourier-transform microwave spectroscopy to give the following hyperfine coupling constants: × aa D = 263.5(25) kHz, D aa DF = −42.7(25) kHz and D aa HF = −244(5) kHz.
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