Abstract

In the present study, ytterbium-169 was produced via the 169Tm(p, n)169Yb nuclear process at the AMIRS (Cyclone-30, IBA, Belgium) cyclotron, irradiating Tm2O3 with proton particles of 15 MeV primary energy and 20 μA current for 20 min. Deposition of Tm2O3 on Cu substrate was carried out via by the sedimentation method. The 543 mg of thulium(III)oxide with 108 mg of ethyl cellulose and 8 mL of acetone were used to prepare a Tm2O3 layer of 11.69 cm2. Yields of about 0.643 MBq 169Yb per μAh were experimentally obtained. 169Yb was separated in 80 ± 5% radiochemical yield using liquid–liquid extraction. Solvent extraction of no-carrier-added 169Yb from irradiated thulium(III)oxide target hydrochloric solution was investigated using di-(2-ethylhexyl)phosphoric acid (HDEHP).

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