Abstract

CuxCo1-xFe2O4 (x = 0.33, 0.67, 1)-reduced graphene oxide (rGO)-thermoplastic polyurethane (TPU) nanocomposites exhibiting highly efficient electromagnetic interference (EMI) shielding were prepared by a melt-mixing approach using a microcompounder. Spinel ferrite Cu0.33Co0.67Fe2O4 (CuCoF1), Cu0.67Co0.33Fe2O4 (CuCoF2) and CuFe2O4 (CuF3) nanoparticles were synthesized using the sonochemical method. The CuCoF1 and CuCoF2 exhibited typical ferromagnetic features, whereas CuF3 displayed superparamagnetic characteristics. The maximum value of EMI total shielding effectiveness (SET) was noticed to be 42.9 dB, 46.2 dB, and 58.8 dB for CuCoF1-rGO-TPU, CuCoF2-rGO-TPU, and CuF3-rGO-TPU nanocomposites, respectively, at a thickness of 1 mm. The highly efficient EMI shielding performance was attributed to the good impedance matching, conductive, dielectric, and magnetic loss. The demonstrated nanocomposites are promising candidates for a lightweight, flexible, and highly efficient EMI shielding material.

Highlights

  • Electromagnetic interference, which is generated by the rapid procreation of electronic and communication technology devices, has become a serious concern in everyday life [1,2]

  • Zahid et al [10] fabricated nanocomposite based on reduced graphene oxide and thermoplastic polyurethane (TPU) matrix and reported a high shielding performance of 53 dB

  • We demonstrated excellent electromagnetic interference (EMI) shielding with MnFe2O4 and reduced graphene oxide (rGO) in a polypropylene matrix [12]

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Summary

Introduction

Electromagnetic interference, which is generated by the rapid procreation of electronic and communication technology devices, has become a serious concern in everyday life [1,2]. The transmission of electromagnetic waves from potential sources, such as mobile phones, radar systems, and different electronic appliances, are cause for interfering with electronic devices, which influences the lifetime and functionality of such electronic instruments [3]. To resolve this problem, the designing of a shielding material endowed with efficient shielding characteristics has become a considerable research interest. The material should contain electrical and magnetic dipoles to be an EM wave absorber [4] In this context, polymer nanocomposites along with magnetic and dielectric nanofillers opened a new pathway due to their lightweight, flexibility, good absorption, low cost, and resistance to corrosion [5]. Sobha et al [11] recorded the EMI shielding efficiency of 31.5 dB by utilizing multi-walled carbon nanotube-based TPU composites

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