Abstract
Mixed crystals of cobalt and zinc were synthesized using 1,3–bis(4–pyridyl)propane (bpp) as bridging ligand and NCS − as anion. Red crystals and blue crystals were obtained. Powder X-ray diffraction patterns showed that the former is in 2D interpenetrated structure, while the latter has the same structure with Zn(NCS)2(bpp). Iron ion was introduced both into the red crystals and blue crystals of the mixed crystals of cobalt with zinc. 57Fe Mossbauer spectrum of the red crystals showed a main doublet of FeII high-spin state at 78 K, while the spectrum of blue crystals did not show FeII high-spin state at 78 K.
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