Abstract
X-ray and neutron powder diffraction were employed to study the crystal and magnetic structures of pseudo-binary Laves-phase compounds (Zr 1− x Mn x )Co 2 and (Zr 1− x Mn x )Co 2.45. It is found that the Zr 0.8Mn 0.2Co 2 compound has the MgCu 2-type cubic structure (space group Fd3m), while Zr 0.64Mn 0.36Co 2.45 and Zr 0.64Mn 0.36Co 2 have the AuBe 5-type (space group F-43m) cubic structure. All compounds are ferromagnets.
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