Critical behavior of the metallic triangular-lattice Heisenberg antiferromagnetPdCrO2

Abstract

We report physical properties of the conductive magnet ${\text{PdCrO}}_{2}$ consisting of a layered structure with a triangular lattice of ${\text{Cr}}^{3+}$ ions $(S=3/2)$. We confirmed an antiferromagnetic transition at ${T}_{\text{N}}=37.5\text{ }\text{K}$ by means of specific heat, electrical resistivity, magnetic susceptibility, and neutron-scattering measurements. The critical behavior in the specific heat persists in an unusually wide temperature range above ${T}_{\text{N}}$. This fact implies that spin correlations develop even at a much higher temperature than ${T}_{N}$. The observed sublinear temperature dependence of the resistivity above ${T}_{\text{N}}$ is also attributed to the short-range correlations among the frustrated spins. While the critical exponent for the magnetization agrees reasonably with the prediction of the relevant model, that for the specific heat evaluated in the wide temperature range differs substantially from the prediction.