Abstract
The rapid growth of electronic technology and communications have led to increase demand for high performance microwave absorbing materials. Ferrites are frequently used to absorb microwaves and protect against electromagnetic contamination. In the present study, β-type hexaferrite samples with different chemical compositions of LiFe11-xCrxO17 (x = 0.0, 0.1, 0.3, and 0.5) have been manufactured through the sol-gel auto-combustion technique. The effect of substituting Cr3+ on its structural, electrical and dielectric characteristics was examined. The XRD evaluation helped to develop a single-phase structure for all samples. The substitution of Cr3+ has changed the structural characteristics. FTIR analysis was used to investigate the vibrational properties of Cr-doped β-type hexaferrite. Two absorption bands in the infrared spectroscopy were used to indicate the tetrahedral and octahedral sites. XPS results revealed the incorporation of every metal ion related to their particular electronic states. The dielectric studies were determined in terms of frequency (1–6 GHz) and every sample behavior was described using the Maxwel-Wagner and Koop theories. Impedance analysis was utilized to study the effects of relaxation time and grain boundaries on the electrical features of the produced nanomaterials. Impedance Cole-Cole plots prove that all samples exhibit non-Debye-type multiple relaxation processes. It was observed that among all the synthesized samples, LiFe10.9Cr0.1O17 has a minimum reflection loss of −37.80 dB at 1.22 GHz. Cr-doped β-type hexaferrite results suggested using and designing hexaferrite-based nanocomposite for high-frequency absorbers in the microwave range.
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