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Abstract
Abstract In a fluoride ion excess CaF 2-type solid solution of formulation M 2+ 1−xM′ 2+α xF 2+αx (α = 1, 2, 3) , the sum of the interstitial fluoride ions n F int and the sum of the vacancies in normal sites n □ can be represented according to general equations y = (mx 3 + λqx)(x 2 + q) : the m and λ parameters depend on structural features, and q is bound to electrical properties. This model allows one to correlate in a continuous way the composition dependence of electrical properties and the progressive extension of clusterization when the substitution rate increases.
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