Abstract
The structural and magnetic properties of the full Heusler alloy Co2FeSi are its key features for practical applications, but the exact structure-function relationship and underlying mechanism still remain unclear. In this detailed study, experiments and simulations clarify the precise correlations between magnetic parameters and the degree of structural ordering. Enhancement of both biaxial anisotropy and atomic ordering are realized with increasing substrate temperature. These findings are helpful for designing advanced spintronic devices with controllable magnetic anisotropy.
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