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Abstract
A procedure for calculating the thermodynamic activity coefficients of oxygen and hydrogen in dilute Na-O-H system melts over the temperature range 300–600°C was suggested. The thermodynamic activity coefficients of hydrogen in liquid sodium calculated by the coordination-cluster model equations were used to determine the equilibrium hydrogen pressure over melts. The calculation results were compared with the experimental partial hydrogen pressures over the Na(excess)-Na2O-NaH system at x O = x H. The calculated values were in qualitative agreement with the experimental data.
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