Abstract
Here, we report a highly efficient cooperative photocatalytic system for the selective oxidation of amines with air. The visible light-assisted adsorption of amines gives rise to a visible light complex on TiO2 that can be self-repaired to safeguard smart photocatalysis. Smart TiO2 photocatalysis works cooperatively with TEMPO catalysis that can perform the visible light-mediated selective oxidation of amines in a swift and recyclable manner. This discovery provides an alternative for addressing environmental challenges by reducing pollutants at the source for oxidative chemical reactions.
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