Abstract

As one of the most important clean fuels, methane plays a significant role in the energy supply system, and its combustion characteristics directly affect the efficiency and emission. In order to avoid the production of a large number of nitrogen oxides, the low temperature combustion associated with cool flame is getting more and more attention. But until now the cool flame characteristics of methane is still unclear, even its existence is controversial. In this work, the property of premixed methane/oxygen cool flame has been experimentally studied in a cylindrical reactor and numerically analyzed using different mechanisms. The effects of pressure, temperature and equivalence ratio on methane cool flame have been investigated experimentally. The experimental results show that the cool flame can be obtained in the range of 0.2–4.8 equivalent ratio. The lower limit of pressure of the cool flame region decreases with the increasing initial temperature. The sensitivity and reaction path have been analyzed through the numerical simulation, which reveals that the bifurcation in CH3 oxidation process has remarkable effects on cool flame formation.

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