Abstract
As you like it: Low-temperature 31P NMR spectroscopic and X-ray crystallographic analyses have revealed that chiral P-spiro triaminoiminophosphorane 1 and 3,5-dichlorophenol (2) selectively assemble into three types of discrete molecular structures, 1⋅[2]n (n=1–3; see picture) depending on the stoichiometry of 2.
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