Abstract
Experimental and theoretical investigations of continuum resonance Raman scattering and related photoinduced, unimolecular dissociation in halogen and interhalogen molecules are discussed. Experimentally observed spectra are simulated using both time-independent and time-dependent theory. The sensitivity of the simulated spectra to small changes in the scattering potentials is demonstrated. The time-dependent approach further allows an estimation of the scattering time for this type of resonance Raman scattering. With iodine chloride, dissociation is monitored by electronic Raman scattering on an iodine atomic transition.
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