Contamination features and health risk of heavy metals in suburban vegetable soils, Yanbian, Northeast China

Abstract

ABSTRACTIn recent years, heavy metal contamination in suburban vegetable soils calls for significant concerns due to the rapid urbanization and industrialization. In present study, 110 suburban vegetable soil samples from Yanbian, Northeast China, were collected. Concentration characteristics, pollution level, health risk, and source identification were evaluated by using different quantitative indices. Concentrations of Pb, Cr, Cu, Ni, Zn, Cd, and As in suburban soils were measured. Mean concentrations of Pb, Cr, Cu, Ni, Zn Cd, and As were 34.9 ± 10.5, 73.5 ± 44.4, 29.6 ± 19.4, 23.4 ± 12.0, 88.5 ± 26.7, 0.16 ± 0.16, and 9.24 ± 3.79 mg/kg, which were showed significantly higher than corresponding background values of Jilin province, respectively. The soils were moderately heavy polluted by Cu and Cd based on the results of geo-accumulated index and pollution indices. The pollution load index indicated that almost all of the study area were middle or heavy polluted, especially in Antu County and Helong City. Children in Yanbian may pose non-carcinogenic and carcinogenic risks with the major exposure pathway of ingestion. Principle component analysis results suggested that Pb, Cu, Zn, and Cd were mainly associated with agricultural activities, Ni and Cr were defined as combined source (lithogenic and anthropogenic), and As was tended to be from excessive application of pesticides and industrial activities.