Abstract

There have been a wide variety of efforts to develop conductive elastomers that satisfy both mechanical stretchability and electrical conductivity, as a response to growing demands on stretchable and wearable devices. This article reviews the important progress in conductive elastomers made in three application fields of stretchable technology: stretchable electronics, stretchable sensors, and stretchable energy harvesters. Diverse combinations of insulating elastomers and non-stretchable conductive materials have been studied to realize optimal conductive elastomers. It is noted that similar material combinations and similar structures have often been employed in different fields of application. In terms of stretchability, cyclic operation, and overall performance, fields such as stretchable conductors and stretchable strain/pressure sensors have achieved great advancement, whereas other fields like stretchable memories and stretchable thermoelectric energy harvesting are in their infancy. It is worth mentioning that there are still obstacles to overcome for the further progress of stretchable technology in the respective fields, which include the simplification of material combination and device structure, securement of reproducibility and reliability, and the establishment of easy fabrication techniques. Through this review article, both the progress and obstacles associated with the respective stretchable technologies will be understood more clearly.

Highlights

  • The demand for stretchable devices has been ever growing since new technology fields like stretchable electronics, intelligent robotics, wearable devices, and body-conformable devices have emerged [1,2,3,4]

  • 1 μm; (d) Conductivity of 3D PDMS–eutectic gallium–indium (PDMS–EGaIn) stretchable conductor under strains of up to 220%; (e) Conductivity variation depending on the number of conductor under strains of up to 220%; (e) Conductivity variation depending on the number of stretching–releasing cycles under different strains

  • The group fabricated polymer light-emitting device (PLED) composed of graphene oxide (GO)–Ag nanowires (AgNWs)–poly(urethane acrylate) (PUA) composite electrodes, a GO–AgNW–PUA composite electrodes, a polymeric emissive layer, and a polyethylenimine (PEI)

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Summary

Introduction

The demand for stretchable devices has been ever growing since new technology fields like stretchable electronics, intelligent robotics, wearable devices, and body-conformable devices have emerged [1,2,3,4]. Keen sensory skins are required to implement advanced robots that can interact well with humans and properly react to the environment without external control [5,6,7] Keeping pace with this growing need for new technology, a wave of searching for new materials that can afford high electrical conductivity and good mechanical elasticity has surged [8,9,10]. Achievements made till but tasks to be solved will be considered

Stretchable Electronics
Stretchable Conductors
Stretchable Field-Effect Transistors and Memories
Stretchable Light-Emitting Diodes
Brief Summary
Stretchable Sensors
Stretchable Strain Sensors
Stretchable
Stretchable Energy Harvesters
Stretchable Solar Cells
Other Stretchable
Findings
Conclusions
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