Concept design, parameter analysis, and thermodynamic evaluation of a novel integrated gasification chemical-looping combustion combined cycle power generation system

Abstract

Integrated gasification chemical-looping combustion (IGCLC) is a potential combustion technology with innate CO2 separation for solid fuels. Coupling this technology with coal-fired power plants is expected to greatly alleviate the high efficiency penalty induced by CO2 capture. This study proposes an innovative system called integrated gasification CLC combined cycle (IGCLCCC) that highly integrates a gasification system, a CLC system, a combined cycle, an ultra-supercritical steam cycle, and a CO2 capture system. In the proposed system, the oxygen-depleted stream from air reactor and flue gas from fuel reactor enter the combined cycle and ultra-supercritical steam cycle, respectively, for power generation. The energy and mass balances of the proposed system are determined by process simulation. The relationship between the performance of subsystems and system efficiency is studied by parameter analysis. Results indicate that the net efficiency penalty (0.3 percentage points) of the proposed system is 4.3 to 13.2 percentage points less than those of the conventional CO2 capture power plants, and the power consumption of specific CO2 capture is minimized to 8.3 kWeh/t. Besides, its net efficiency is as high as 45.0%, which is comparable to that of the natural gas combined cycle power plant with a 90% CO2 capture rate. This work provides a new sight into the design of the low-carbon and efficient power generation system.