Concentration, Spatial Distribution, Contamination Degree and Human Health Risk Assessment of Heavy Metals in Urban Soils across China between 2003 and 2019-A Systematic Review.

Shuangmei Tong,Muyesaier Tudi,Linsheng Yang,Li Wang,Hairong Li

doi:10.3390/ijerph17093099

Abstract

This study provides an overview of the studies of heavy metal pollution regarding As, Cd, Cr, Hg, Pb, Cu, Zn and Ni in the urban soils throughout 71 cities of China, based on data from online literature, during the period 2003–2019. The concentrations, spatial distributions, contamination degrees and health risks of heavy metals in the urban soils were evaluated. The results demonstrated that the mean values of eight heavy metals all exceeded the soil background values in China, and the kriging interpolation method showed that the hot-spot cities with heavy metal contamination in urban soils were mainly concentrated in the southwest, southcentral, southeast coast, northcentral and northwest regions of China. The geoaccumulation index (Igeo) indicated that Hg and Cd were at moderate contamination levels and that the levels of the other six metals did not appear contamination. The pollution index (PI) showed that Cd and Hg reached high contamination levels, and the other metals reached moderate contamination levels. The integrated pollution index (IPI) and potential ecological risk index (PRI) indicated that the integral urban soils in the study areas ranked high contamination levels and moderate ecological risk degree, respectively, and Cd and Hg should be labeled as priority metals for control in the urban soils around China. The human health risk assessments for the heavy metals indicated that ingestion was the dominant exposure pathway for having adverse effects on human health. The mean Hazard index (HI) values of eight heavy metals all showed that adverse effects on human health were unlikely, and the mean carcinogenic (CR) values of As, Cr and Ni for children and adults all suggested an acceptable carcinogenic risk to human beings. In addition, children exposed to these heavy metals faced more serious non-carcinogenic and carcinogenic health threats compared to adults. The results could provide valuable information for demanding the better control of heavy metal pollution and mitigation of the adverse effects on residents by environmental regulators in national urban regions.

Highlights

As a crucial component of urban ecosystems, soil plays a principal role in biochemical transformation, the cycling of elements, supporting plants and many recreational activities
The hot-spot cities for heavy metals in urban soils were mainly concentrated in the southwest, southcentral, southeast, east coast, northwest and northcentral regions of China, which should be labeled as priority regions for controlling heavy metal contamination
According to the integrated pollution index (IPI) and potential ecological risk index (PRI) values (Figure 5), the high contamination and ecological risk regions were mainly concentrated in the southwest, south center, north center, east and east coast regions of China, while the cities were mainly located in Kashi, Changsha, Shangluo, Tongchuan, Lvliang, Jinchang, Luoyang, Baoji, Ganzhou, Shenyang and Baiyin

Summary

Objectives

The main objectives of this study are (a) to determine the concentrations and spatial distribution of As, Cd, Cr, Hg, Pb, Cu, Zn and Ni—eight heavy metals—in urban soils; (b) to evaluate the pollution characteristics of the heavy metals using the geoaccumulation index (Igeo), pollution index

Methods

Results

Conclusion