Abstract
Comprehensive SummaryContinuous‐flow techniques have promoted the development of synthetic chemistry due to advantages such as outstanding mass/heat transfer, on‐demand scalability, improved safety, precise regulation on reaction parameters, etc. Recently, the combination of flow polymerization with computer science has gained considerable interests, leading to a variety of cutting‐edge synthetic techniques. This review summarizes emerging achievements realized via the integration of computer science and living flow polymerizations, including 1) high‐throughput living polymerizations in flow, 2) programmable regulations of dispersity profile, sequence and topology for polymers, 3) modular design with online monitoring, as well as 4) self‐optimized living polymerizations in flow. We expect that this summary will furnish informative knowledge to scientists in related directions and inspire new ideas to further empower on‐demand polymer engineering with modern techniques.
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