Abstract
The photodissociation of CH 2Cl is studied by the ion imaging technique. At 235–243 nm, Cl photofragments are produced via the simultaneous excitation of the perpendicular (1 2 A 1←1 2 B 1) and parallel (2 2 B 1←1 2 B 1) electronic transitions. The relative populations and translational energy distributions of Cl fragments generated via each transition are extracted. H-atom products, which are detected in a one-color experiment at 243.1 nm, exhibit an angular distribution characteristic of perpendicular transitions only. They may be produced via excitation to the valence 1 2 A 1 and/or Rydberg 2 2 A 1 (3s) states.
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