Comparison of Aerosol Optical Properties Between Two Nearby Urban Sites in Beijing, China

Abstract

This study compares the aerosol optical properties measured by CE318 sunphotometers at the Institute of Atmospheric Physics and the Chinese Academy of Meteorological Sciences in Beijing between January 2013 and July 2015 to provide the framework to quantify the spatial and temporal variability of aerosol properties. Aerosol optical parameters included extinction (scattering plus absorption) aerosol optical depth (EAOD), extinction Angstrom exponent (EAE), columnar water vapor (CWV), absorption aerosol optical depth (AAOD), absorption Angstrom exponent (AAE), extinction aerosol optical depth of fine particles (EAODf), extinction aerosol optical depth of coarse particles (EAODc), real parts of the refractive index (REFR), imaginary parts of the refractive index (REFI), single scattering albedo (SSA), asymmetry factor (ASYM), size distribution, and sphericity fraction. Comparison of aerosol optical properties using the simultaneous observations between two sites showed that correlation coefficients were larger than or equal to 0.98 for EAOD, EAE, and CWV, but smaller than or equal to 0.90 for AAOD, REFR, REFI, and SSA; the percentage differences for most of the parameters were less than 2%, but for EAODf were relatively large, ranging from 4.35 to 6.45%; the mean size distributions simultaneously showed bi-modal patterns, with two peak volumes at the radii of 0.15 and 2.94 μm; two kinds of tri-peak model were apparent during the study period; a case of EAODs at 440 nm differing by more than 0.2 between the two sites reflected the effect of local aerosol pollution. Comparison of aerosol characterization inferred by absorption properties using all the inversion data showed that classification using EAE, AAE, and sphericity fraction indicated the main aerosol type was “U/IB the volume size distribution retrievals binned by AAE exhibited coarse mode particles became dominant as AAE increased to 2.0; the SSA retrievals binned by AAE demonstrated SSA transitioned from spectra representing dust to U/IB averaged SSA for all the retrievals and SSA data partitioned by the EAE and η 675 nm suggested there were more absorbing aerosols at IAP. The results of the study will be beneficial in validating satellite observations and model simulation results, providing more accurate input parameters for model simulations.