Abstract

Human health is strongly affected by the concentration of fine particulate matter (PM2.5). The need to forecast unhealthy conditions has driven the development of Chemical Transport Models such as Community Multi-Scale Air Quality (CMAQ). These models attempt to simulate the complex dynamics of chemical transport by combined meteorology, emission inventories (EI’s), and gas/particle chemistry and dynamics. Ultimately, the goal is to establish useful forecasts that could provide vulnerable members of the population with warnings. In the simplest utilization, any forecast should focus on next day pollution levels, and should be provided by the end of the business day (5 p.m. local). This paper explores the potential of different approaches in providing these forecasts. First, we assess the potential of CMAQ forecasts at the single grid cell level (12 km), and show that significant variability not encountered in the field measurements occurs. This observation motivates the exploration of other data driven approaches, in particular, a neural network (NN) approach. This approach makes use of meteorology and PM2.5 observations as model predictors. We find that this approach generally results in a more accurate prediction of future pollution levels at the 12 km spatial resolution scale of CMAQ. Furthermore, we find that the NN is able to adjust to the sharp transitions encountered in pollution transported events, such as smoke plumes from forest fires, more accurately than CMAQ.

Highlights

  • Fine particulate matter air pollution (PM2.5 ) is an important issue of public health, for the elderly and young children

  • In our present assessment of the current operational Community Multi-Scale Air Quality (CMAQ) forecast model (Version 4.6), we differ from the regional studies above in the following ways: Firstly, in addition to the 1200 UTC forecast, we evaluated the 0600 UTC forecast for the same period to determine if release time affects the CMAQ

  • This study showed the importance of planetary boundary layer (PBL) height dynamics and meteorological factors that motivated the choice of meteorological forecast inputs used during the neural network (NN) development

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Summary

Introduction

Fine particulate matter air pollution (PM2.5 ) is an important issue of public health, for the elderly and young children. The study by Pope et al suggests that exposure to high levels of PM2.5 is an important risk factor for cardiopulmonary and lung cancer mortality [1,2]. In addition to local emission sources, pollution events can be the result of aerosol plume transport and intrusion into the lower troposphere. When there is a potential high pollution event, the local air quality agencies must alert the public, and advise the population on proper safety measures, as well as direct the reduction of emission producing activities. Accurately measuring and predicting fine particulate levels is crucial for public safety

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