Abstract

Abstract. This is a comment on the review by Korolev and Leisner (2020, hereafter KL2020). The only two laboratory/field studies ever to measure the breakup in ice–ice collisions for in-cloud conditions were negatively criticised by KL2020, as were our subsequent theoretical and modelling studies informed by both studies. First, hypothetically, even without any further laboratory experiments, such theoretical and modelling studies would continue to be possible, based on classical mechanics and statistical physics. They are not sensitive to the accuracy of lab data for typical situations, partly because the nonlinear explosive growth of ice concentrations continues until some maximum concentration is reached. To a degree, the same final concentration is expected regardless of the fragment number per collision. Second, there is no evidence that both lab/field observational studies characterising fragmentation in ice–ice collisions are either mutually conflicting or erroneous such that they cannot be used to represent this breakup in numerical models, contrary to the review. The fact that the ice spheres of one experiment were hail sized (2 cm) is not a problem if a universal theoretical formulation, such as ours, with fundamental dependencies, is informed by it. Although both lab/field studies involved head-on collisions, rotational kinetic energy for all collisions generally is only a small fraction of the initial collision kinetic energy (CKE) anyway. Although both lab/field experiments involved fixed targets, that is not a problem since the fixing of the target is represented via CKE in any energy-based formulation such as ours. Finally, scaling analysis suggests that the breakup of ice during sublimation can make a significant contribution to ice enhancement in clouds, again contrary to the impression given by the review.

Highlights

  • The literature of secondary ice production (SIP) was recently reviewed by Korolev and Leisner (2020, hereafter KL2020)

  • It is commendable that their review attempts to reinvigorate laboratory observations of the various types of fragmentation of ice, research that has in the last decade been oriented towards heterogeneous ice nucleation

  • Even if the available data were unreliable or unrepresentative of natural clouds, which is not the case (Sect. 4), our stand-alone theoretical and modelling studies would, still have been possible, since they are based on classical mechanics of collisions and statistical physics: 1. Yano and Phillips (2011) and Yano et al (2016) delineated the timescale of the explosive growth of ice concentrations and the conditions for such instability in terms of dimensionless parameters that provide a phase space of the system

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Summary

Introduction

The literature of secondary ice production (SIP) was recently reviewed by Korolev and Leisner (2020, hereafter KL2020). Theory of Yano and Phillips (2011) to treat the breakup in graupel–snow collisions, estimating that c ≈ 10 They found this was consistent with an increase by an order of magnitude of average ice concentrations in about an hour, as predicted by the detailed cloud simulation. Phillips et al (2017a) created a formulation for the number of fragments from any collision of two ice particles as a function of their sizes, velocities, temperature and morphology It was based on principles of theoretical statistical physics considering energy conservation at the particle scale. An alternative type of SIP from the collision of a raindrop with a more massive ice particle was represented (Mode 2) The formulation for both modes was applied in a detailed bin microphysics parcel simulation and shown to reproduce aircraft observations of cloud glaciation for a tropical convective case. Note that the SIP mechanism discussed by Phillips et al (2018) has no connection whatsoever with the topic that it was erroneously cited for by KL2020, namely the breakup in ice–ice collisions (see the Corrigendum)

The breakup in ice–ice collisions
Sublimational breakup
Findings
Conclusions

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