Comment on acp-2022-796

Abstract

<strong class="journal-contentHeaderColor">Abstract.</strong> The Amazon rainforest routinely experiences intense and long-lived biomass burning events that result in smoke plumes that cover vast regions. The spatial and temporal extent of the plumes, and the complex pathways through which they interact with the atmosphere, has proved challenging to measure and gain a representative understanding of smoke impacts on the Amazonian atmosphere. In this study we use multiple collocated satellite sensors onboard AQUA and TERRA platforms to study the underlying smoke-cloud-radiation interactions during the diurnal cycle. An 18-year timeseries for both morning and afternoon overpasses is constructed providing collocated measurements of aerosol optical depth (column integrated aerosol extinction, AOD), cloud properties, top-of-atmosphere radiative fluxes, precipitation, and column water-vapour content from independent sources. The long-term timeseries reduces the impact of interannual variability and provides robust evidence that smoke significantly modifies the Amazonian atmosphere. Low loadings of smoke (AOD &le; 0.4) enhance convective activity, cloudiness and precipitation, but higher loadings (AOD &gt; 0.4) strongly suppress afternoon convection and promote low-level cloud occurrence. Accumulated precipitation increases with convective activity but remains elevated under high smoke loadings suggesting fewer but more intense convective cells. Contrasting morning and afternoon cloud responses to smoke are observed, in-line with recent simulations. Observations of top-of-atmosphere radiative fluxes support the findings, and show that the response of low-level cloud properties and cirrus coverage to smoke results in a pronounced and consistent increase in top-of-atmosphere outgoing radiation (cooling) of up to 50 Wm^-2 for an AOD perturbation of +1.0. The results demonstrate that smoke strongly modifies the atmosphere over the Amazon via widespread changes to the cloud-field properties. Rapid adjustments work alongside instantaneous radiative effects to drive a stronger cooling effect from smoke than previously thought, whilst contrasting morning/afternoon responses of liquid and ice water paths highlight a potential method for constraining aerosol impacts on climate. Increased drought susceptibility, land-use change, and deforestation will have important and widespread impacts to the region over the coming decades. Based on this analysis, we anticipate further increases in anthropogenic fire activity to be associated with an overall reduction in regional precipitation, and a negative forcing (cooling) on the Earth&rsquo;s energy budget.