Abstract
We show the synthetic procedure of colored magnetic films composed of Prussian blue analog-based magnets and their magneto-optical effects in the visible region. Magnetic thin films of M 3 II [ Cr III ( CN ) 6 ] 2 · z H 2 O (M = Co, Ni, Cu) are prepared on transparent Nafion membrane by an ion-exchange process and these films exhibit Faraday effect due to d–d transition of M II. The film-type of ( Fe x I Cr 1 - x II ) 3 [ Cr III ( CN ) 6 ] 2 · 15 H 2 O is electrochemically prepared by reducing aqueous solutions containing three compounds of K 3[Cr(CN) 6], CrCl 3, and FeCl 3. These films display magnetization-induced second harmonic generation below Curie temperature.
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