Abstract
Coherent rotational dynamics of gas-phase molecules induced by the excitation with an intense nonresonant ultrafast laser field is discussed. In particular, utilities of quantum-state resolved spectroscopic probe after the nonadiabatic rotational excitation (NAREX) by the ultrafast pulse(s) are described with an example of double-pulse excitation experiments on NO, which provide detailed information on excitation pathways in NAREX. Future prospects of the present method are briefly discussed.
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