Abstract

The light scattering from a single resonant molecule, or nano-sized particle located near the tip of an apertureless scanning near-field microscope is studied, and different regimes of scattering are analyzed. The tip enhances the external field, and serves as an efficient transmission `antenna' for the molecular dipole oscillations. The light scattering occurs via two channels: direct scattering from the tip, and tip-mediated molecular scattering. The total detected intensity of the scattered light shows interference of the channels, which we suggest to use for efficient near-field microscopy. At certain detunings from resonances the scanning signal experiences spatial narrowing similar to that one observed in two-photon microscopy, thus allowing for sub-nanometer resolution.

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