Abstract
This paper presents the results of experimental investigations of a series of conformationally inhomogeneous compounds with polarization sensitive coherent active (anti-Stokes) Raman scattering spectroscopy (PS CARS). Interpretation of vibrational spectra is refined and spectroscopic parameters are determined of resonances of complex spectral band ofn-penthane (bands at 868 and 841 cm'') 5 2-ethinyle 1 (bands at 949 and 910 cm ) which were not resolved previously with use of spontaneous Raman scattering spectroscopy (SRS). Thereby the principle of holographic spectroscopy was realized and tested in the full scale. 1.
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