Abstract
We report the observation of coherent control of the ionization rate in four-photon resonant, five-photon ionization schemes in Kr and Xe. The intermediate resonance is excited via different interfering channels involving four-photon absorption of the fundamental laser frequency ( ionization) as well as one third harmonic and one fundamental frequency photon absorption ( excitation), a particular aspect of the scheme being that interference occurs at a virtual level. By varying the relative phase of the two electromagnetic fields, a large modulation depth has been observed which is due to the chosen non-linear excitation scheme. In the Xe excitation experiment the interference between the different channels could be additionally probed through the modulation of the third-harmonic signal.
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