Abstract
The feasibility of laser control over branching unimolecular reactions, and laser catalysis of bimolecular reactions is investigated. Laser control in unimolecular reactions is being discussed using a two-colour excitation scheme. It is shown that specific products are obtained in preference to others as a result of interference between final states produced in two different excitation (and dissociation) routes. Computational results on the I*/I branching ratios in the photodissociation of CH3I, illustrating the degree of control achievable are presented.
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