Abstract

Magnetoactive polymer composites (MAPCs) are materials composed of a polymer matrix embedded with magnetic particles that mechanically respond to external magnetic fields. MAPCs can be programmed to be adjusted remotely without physical interventions using a magnetic field to generate the desired response; therefore, MAPCs are being actively explored for their applications in remote sensing, soft robotics, electronics, and biomedical areas. In this work, novel MAPCs were synthesised comprising polyvinyl alcohol (PVA) as the matrix and cobalt iron oxide (CoFe2O4) nanoparticles as the magnetic component with varying concentrations (i.e., 1.25%, 2.5%, and 5%). MAPCs were synthesised using the solution casting technique, and field emission scanning electron microscopy (FE-SEM) and x-ray diffraction (XRD) results revealed the successful integration of CoFe2O4 nanoparticles within the polymer matrix. The synthesised MAPC films were also characterised for their chemical, thermal, magnetic, and biological properties. The incorporation of CoFe2O4 nanoparticles resulted in an improved magnetic response, with improvements in these properties with increasing CoFe2O4 content. PVA/5% CoFe2O4 revealed toxicity and requires further investigation of using these materials with higher CoFe2O4 concentrations. The magnetic response and biological properties of the PVA/CoFe2O4 MAPCs revealed their potential uses for remote actuation and sensing in the biomedical sector.

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