Abstract

The contactless coalescence of a droplet is of paramount importance for physical and industrial applications. This paper describes a coalescence method to be used mid-air via acoustic levitation using an ultrasonic phased array system. Acoustic levitation using ultrasonic phased arrays provides promising lab-on-a-drop applications, such as transportation, coalescence, mixing, separation, evaporation, and extraction in a continuous operation. The mechanism of droplet coalescence in mid-air may be better understood by experimentally and numerically exploring the droplet dynamics immediately before the coalescence. In this study, water droplets were experimentally levitated, transported, and coalesced by controlled acoustic fields. We observed that the edges of droplets deformed and attracted each other immediately before the coalescence. Through image processing, the radii of curvature of the droplets were quantified and the pressure difference between the inside and outside a droplet was simulated to obtain the pressure and velocity information on the droplet’s surface. The results revealed that the sound pressure acting on the droplet clearly decreased before the impact of the droplets. This pressure on the droplets was quantitatively analyzed from the experimental data. Our experimental and numerical results provide deeper physical insights into contactless droplet manipulation for futuristic lab-on-a-drop applications.

Highlights

  • The acoustic levitation [1,2] of droplets is a promising tool for contactless fluid manipulation for lab-on-a-drop applications [3,4,5,6,7,8] by achieving droplet levitation, transportation, coalescence, mixing, separation, evaporation, and extraction in a single operation

  • We observed that the edges of the droplets deformed and attracted each other immediately before the coalescence by quantifying the radii of curvature of droplets via in-house image processing

  • The symmetrical droplet shape contributed significantly to the coalescence of droplets. This may be have due to the interaction of droplets and sound pressure field when the droplets were closely approaching with less than a millimeter of the distance between them

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Summary

Introduction

The acoustic levitation [1,2] of droplets is a promising tool for contactless fluid manipulation for lab-on-a-drop applications [3,4,5,6,7,8] by achieving droplet levitation, transportation, coalescence, mixing, separation, evaporation, and extraction in a single operation. A sample can be suspended using the acoustic radiation force acting on the object [9]. This method enables contactless treatment to avoid the contamination, absorption, and heterogeneous nucleation through the wall effect [2]. Marzo et al [11] demonstrated a novel technique for particle manipulation using an ultrasonic phased array system. After the successful merging of droplets, a single droplet was effectively mixed by inducing the 6th mode oscillation on its surface. Hasegawa et al [14] observed that that the internal flow field induced by the mode oscillation promoted the mixing performance with varying Reynolds number

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