Abstract
Interface engineering is an effective strategy for improving the activity of catalysts in electrocatalytic oxygen evolution reaction (OER). Herein, Co3 O4 supported on β-Mo2 C with different interfaces were investigated for electrocatalytic OER. The morphological diversity of β-Mo2 C supports allowed different Co3 O4 -Mo2 C interactions. Various techniques characterized the composition and microstructure of the interface in the composites. Due to the strong interaction between Co3 O4 nanoparticles and β-Mo2 C nanobelts with opposing surface potentials, compact interface was observed between Co3 O4 active species and β-Mo2 C nanobelt support. The compact interface enhanced the conductivity of the material and also regulated the interfacial electron redistribution of Mo and Co atoms, promoting the charge transfer process during OER. In addition, the surface loading of Co3 O4 can effectively improve the hydrophilicity of the surface. β-Mo2 C has the capability in dissociating H2 O molecules. Thus, an example has been carefully demonstrated for interface engineering in electrocatalytic OER.
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