CO2 retention in high-pressure/high-temperature reservoirs of the Yinggehai Basin, northwestern South China Sea

Abstract

Global industry drillings targeted at deep-burial hydrocarbons have renewed the record of maximum sustainable overpressure in sedimentary basins. However, the influence of extremely high overpressure on natural fluid accumulation and artificial waste sequestration is not yet completely understood. To better understand the motion characteristics of the highly overpressured CO2-rich fluid, the CO2 retention capacity was quantified, and the CO2-rich fluid motion trails were evaluated in an ideal natural laboratory in the Yinggehai Basin. The hydraulic sealing capacity was higher than the capillary sealing capacity in the highly overpressured stratum. Relative to the situations of no breach or solely breached by capillary failure, the superposition of capillary and hydraulic failures resulted in the caprock integrity breakage by faults (or fractures), diapirs, and pipes. Meanwhile, the high expulsion flux of CO2-rich fluid caused the consumption of chlorite to generate illite in the caprock of dual-breached fields. The CO2-rich fluid flux of capillary invasion was limited by the inherently low permeability of caprock, which may be insufficient for a dramatic change of hydrogen ions or electron activities to induce remarkable chlorite dissolution in the caprock of the sole-breached field.