Abstract

We report here a new double-cage endohedral Ge cluster, [Co2@(Ge17Ni)]4-, fused through two [Co@(Ge9Ni)] moieties with a shared Ni-Ge edge. This ternary Co-Ge-Ni species not only represents the first double-cage example of an 18-vertex Zintl cluster, but also fills in the missing link of the edge fusion model in the double-cage systems.

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