CO2 Capture by Aqueous Solution Containing Mixed Alkanolamines and Diethylene Glycol in a Rotating Packed Bed

Abstract

In this study, an effective absorbent, 23.5% diethylenetriamine (DETA)/19.6% piperazine (PZ)/37.7% diethylene glycol (DEG)/19.2% H2 O, was proposed to capture CO2 from a nitrogen gas stream containing 10% of CO2 in a rotating packed bed (RPB). The addition of DEG could improve the solubility of PZ in absorbent, and there was no precipitation observed in CO2 - rich solution after CO2 absorption for the proposed absorbent. The regeneration energy could be reduced because the heat capacity and vapor pressure of DEG are lower than that of water. The higher gas-liquid contact area and mass transfer rate as well as the smaller size were observed in a RPB as compared with a packed bed to achieve the same CO2 capture efficiency.