Abstract

The dynamics of multi-photon induced fragmentation of N2 has been investigated in XUV-pump/XUV-probe experiments at the Free-Electron Laser in Hamburg (FLASH) by recording the ion kinetic energy release(KER) and angular distributions for various dissociation- and Coulomb-explosion channels as a function of the pump-probe delay-time.

Highlights

  • Synopsis The dynamics of multi-photon induced fragmentation of N2 has been investigated in XUVpump/XUV-probe experiments at the Free-Electron Laser in Hamburg (FLASH) by recording the ion kinetic energy release(KER) and angular distributions for various dissociation- and Coulomb-explosion channels as a function of the pump-probe delay-time

  • The interaction of very intense XUVradiation with molecules is governed by multiple ionization and dissociation initiated by fewphoton absorption

  • In the experiment we used very intense (~ 1012 W/cm2), ultra-short (~ 30 fs) light-pulses (28 eV) delivered by FLASH in combination with a reaction microscope equipped with a XUV split-and-delay mirror

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Summary

Introduction

Synopsis The dynamics of multi-photon induced fragmentation of N2 has been investigated in XUVpump/XUV-probe experiments at the Free-Electron Laser in Hamburg (FLASH) by recording the ion kinetic energy release(KER) and angular distributions for various dissociation- and Coulomb-explosion channels as a function of the pump-probe delay-time. *Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai, 201210, China † Max-Planck-Institut für Kernphysik, Heidelberg, 69117, Germany §Max-Planck-Institut für Quantenoptik, Garching, 85748, Germany ||Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, Sendai, 980-8577, Japan

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